Through a collaborative effort involving the Universities of Groningen and Amsterdam in the Netherlands, along with Italy's European Laboratory for Non-Linear Spectroscopy, scientists have significantly advanced photoclick chemistry. They enhanced the reactivity of the photoclick compound used in th
in the Netherlands, along with Italy’s European Laboratory for Non-Linear Spectroscopy, scientists have significantly advanced photoclick chemistry. They enhanced the reactivity of the photoclick compound used in the widely-utilized PQ-ERA reaction through strategic molecular substitution., the flagship journal of the Royal Society of Chemistry, they report a superb photoreaction quantum yield, high reaction rates, and notable oxygen tolerance.
At the University of Amsterdam, Michiel Hilbers and Wybren Jan Buma of the Molecular Photonics group contributed to the research of which the synthetic and reaction characterization part was conducted in the laboratories of Wiktor Szymanski and Nobel laureate Ben Feringa at the University of Groningen.Photoclick chemistry is a light-activated variety of click chemistry , a set of elegant and efficient chemical reaction methods that couple dedicated molecular units to yield desired products.
Nanosecond time-resolved spectroscopic studies and quantum chemical studies in the Amsterdam Molecular Photonics group combined with femtosecond time-resolved spectroscopic studies performed in Florence provided a fundamental understanding of this specific photoclick chemistry. The investigations show that the substitution significantly increases the population of the reactive triplet state during excitation of 3-thiophene PQs.
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